Chamond sat for his county five times and brought his sons into Parliament for the nearby borough of Bodmin.
Chamond served on a number of local commissions and undertook some ad hoc tasks, such as, in 1574, conducting a survey of forts and castles in Cornwall, and reporting to the Privy Council on measures to strengthen the defences. On a number of occasions he was accused of bribery, and of suborning juries, and was involved in disputes over property and rights of hunting and fishing.
He died 11 Apr. 1599. In his will, made in 1596, he provided legacies for his children and servants. Twenty shillings were bequeathed to the poor in each of the parishes of Launcells, Stratton and Kilkhampton.
